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I don't think of Harry Potter or lunatic, personally. I think of a hippy-ish girl. :b I've never personally known a Luna, but I watched a soap opera for several years that had a character named Luna who was a bit "eccentric", hippy-ish, somewhat ditzy, but very sweet and lovable (One Life to Live, btw). I would definitely consider it for a pet because I do like it a lot, though not necessarily enough to use on a child (but I wouldn't discourage its use on a real child, either).

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Don't care for the Loona spelling at all. That really makes me think of "loony" or Looney Tunes. I don't see Luna getting hugely popular, no, though it might get used a little more in the upcoming years. Luna & Elsa or Luna & Kaia would definitely work for sisters. I'm not feeling all 4 together, though.